孙治湖，博士，研究员，博士生导师。长期致力于应用和发展原位同步辐射X射线吸收谱学(XAFS)技术，是全国同步辐射XAFS专业委员会委员。利用原位XAFS技术研究了一系列金属和半导体纳米颗粒和纳米团簇的成核、生长、转化、结构演变等动态过程的内在机制等。近年来，更是针对当前催化科学领域迫切需要解决的问题，发展operando XAFS实验技术和分析方法，对工作状态下的催化剂在真实的催化反应条件下的动态结构开展operando研究。还研究了一系列半导体量子点和二维纳米材料的结构与性能之间的相互关系等。

作为项目负责人共主持了7项国家自然科学基金，包括1项基金委大科学装置联合基金重点项目、5项面上项目和1项青年基金项目，并主持和参与了多项其他基金项目。近10年来发表论文90余篇，其中以第一/通讯作者发表论文40余篇，I区论文30多篇，包括Nature Commun.、JACS、Angew. Chem.等高水平论文。论文被引10500余次，H因子48。

 

学习经历

1993. 9 – 1997. 7   中国科学技术大学 | 材料物理专业 | 理学学士学位

1997. 9 – 2000. 6   中国科学技术大学 | 理论物理 | 理学硕士学位

2000. 9 – 2003.12  中国科学技术大学 | 核技术及应用 | 工学博士学位

 

工作经历

2007.10 – 2009. 9  日本产业技术总合研究所(AIST) | 博士后

2004. 1 – 2010. 6  中国科学技术大学 | 国家同步辐射实验室 | 助理研究员

2010. 6 – 2022.11  中国科学技术大学 | 国家同步辐射实验室 | 副研究员

2022.11–  现在      中国科学技术大学 | 国家同步辐射实验室 | 研究员

 

研究方向

X射线谱学技术及其原位应用

催化材料形成过程和反应机制研究

功能材料的构效关系研究

 

发表论文

[1] R. Xu, Y. Pan, Q. Guan, L. Xu, F. Song, J. Ma, M. Ge, W. Chen, Y. Liu, Q. Ji, C. Wang, J. Yuan, X. Chen, Z. Sun, Electronic metal-support interactions between zeolite and confined platinum-tin nanoalloy boosting propane dehydrogenation, Applied Catalysis B: Environment and Energy, 358 (2024) 124438.

[2] R.C. Xu, H.M. Li, L.X. Xu, Y. Pan, M. Ge, C. Wang, Z.H. Sun, Interfacial synergy between PtCo nanoparticles and CoO for efficient ammonia borane hydrolysis, Chem. Eng. J., 479 (2024) 147773.

[3] C.-H. Gu, Y. Pan, T.-T. Wei, A.-Y. Zhang, Y. Si, C. Liu, Z.-H. Sun, J.-J. Chen, H.-Q. Yu, Upcycling waste sewage sludge into superior single-atom Fenton-like catalyst for sustainable water purification, Nature Water, 2 (2024) 649-662.

[4] X.H. Zhang, Z.H. Sun, R. Jin, C.W. Zhu, C.L. Zhao, Y. Lin, Q.Q. Guan, L.N. Cao, H.W. Wang, S. Li, H.C. Yu, X.Y. Liu, L.L. Wang, S.Q. Wei, W.X. Li, J.L. Lu, Conjugated dual size effect of core-shell particles synergizes bimetallic catalysis, Nature Communications, 14 (2023) 530.

[5] L.X. Xu, Y. Pan, H.M. Li, R.C. Xu, Z.H. Sun, Highly active and water-resistant Lanthanum-doped platinum-cobalt oxide catalysts for CO oxidation, Applied Catalysis B-Environmental, 331 (2023) 122678.

[6] L. Xu, W. Zhou, C. Yang, H. Su, Q. Liu, Z. Sun, S. Wei, Synchrotron radiation XAFS applications in the in situ measurement for energy catalysis, SCIENTIA SINICA Chimica, 53 (2023) 2117-2144.

[7] Z.H. Sun, G.Y. Feng, X.S. Liu, Construction of Hefei advanced light facility begins, The Innovation, 4 (2023) 100514.

[8] X.Y. Liu, Q.Q. Gu, Y.F. Zhang, X.Y. Xu, H.W. Wang, Z.H. Sun, L.A. Cao, Q.M. Sun, L.L. Xu, L.L. Wang, S. Li, S.Q. Wei, B. Yang, J.L. Lu, Atomically Thick Oxide Overcoating Stimulates Low-Temperature Reactive Metal-Support Interactions for Enhanced Catalysis, Journal of the American Chemical Society, 145 (2023) 6702-6709.

[9] H.M. Li, W.X. He, L.X. Xu, Y. Pan, R.C. Xu, Z.H. Sun, S.Q. Wei, Synergistic interface between metal Cu nanoparticles and CoO for highly efficient hydrogen production from ammonia borane, Rsc Advances, 13 (2023) 11569-11576.

[10] Q.Y. Wang, Y. Xiao, S.K. Yang, Y.D. Zhang, L.H. Wu, H.B. Pan, D.W. Rao, T. Chen, Z.H. Sun, G.M. Wang, J.F. Zhu, J. Zeng, S.Q. Wei, X.S. Zheng, Monitoring Electron Flow in Nickel Single-Atom Catalysts during Nitrogen Photofixation, Nano Letters, 22 (2022) 10216-10223.

[11] Y. Pan, L.X. Xu, W.X. He, H.M. Li, W. Chen, Z.H. Sun, Optimizing the synergy between alloy and alloy-oxide interface for CO oxidation in bimetallic catalysts, Nanoscale, 14 (2022) 7303-7313.

[12] Y.Y. Liu, L. Cai, Q.Q. Ji, C. Wang, Z.Y. Liu, L.Y. Lv, B. Tang, H.L. Duan, F.C. Hu, H.J. Wang, N. Li, Z.H. Sun, W.S. Yan, Operando Identification of Dual Active Sites in Ca2IrO4 Nanocrystals with Yttrium Substitutions Boosting Acidic Oxygen Evolution Reaction, Acs Energy Letters, (2022).

[13] X.Y. Liu, J. Luo, H.W. Wang, L. Huang, S.S. Wang, S. Li, Z.H. Sun, F.F. Sun, Z. Jiang, S.Q. Wei, W.X. Li, J.L. Lu, In Situ Spectroscopic Characterization and Theoretical Calculations Identify Partially Reduced ZnO1-x/Cu Interfaces for Methanol Synthesis from CO2, Angew. Chem. Int. Ed., 61 (2022).

[14] W.X. He, X. Zhang, K. Zheng, C.Q. Wu, Y. Pan, H.M. Li, L.X. Xu, R.C. Xu, W. Chen, Y. Liu, C. Wang, Z.H. Sun, S.Q. Wei, Structural Evolution of Anatase-Supported Platinum Nanoclusters into a Platinum-Titanium Intermetallic Containing Platinum Single Atoms for Enhanced Catalytic CO Oxidation, Angew. Chem. Int. Ed., (2022) e202213365.

[15] H.L. Duan, G.N. Li, H. Tan, C. Wang, Q. Li, C.C. Liu, Y.W. Yin, X.G. Li, Z.M. Qi, W.S. Yan, Sulfur-vacancy-tunable interlayer magnetic coupling in centimeter-scale MoS2 bilayer, Nano Research, 15 (2022) 881-888.

[16] S. Chen, B.B. Gong, J. Gu, Y. Lin, B. Yang, Q.Q. Gu, R. Jin, Q. Liu, W.X. Ying, X.X. Shi, W.L. Xu, L.H. Cai, Y. Li, Z.H. Sun, S.Q. Wei, W.H. Zhang, J.L. Lu, Dehydrogenation of Ammonia Borane by Platinum-Nickel Dimers: Regulation of Heteroatom Interspace Boosts Bifunctional Synergetic Catalysis, Angew. Chem. Int. Ed., 61 (2022) e202211919.

[17] S.Y. Wang, L. Huang, C.Y. Liu, W.X. He, Z.X. Long, Y. Pan, Z.H. Sun, Promoting Effect of Co(OH)2 for Supported Pt Nanocatalysts toward Catalytic Hydrolysis of Ammonia Borane, Chinese Journal of Chemical Physics, (2021).

[18] L.L. Wang, C.W. Zhu, M.Q. Xu, C.L. Zhao, J. Gu, L.N. Cao, X.H. Zhang, Z.H. Sun, S.Q. Wei, W. Zhou, W.X. Li, J.L. Lu, Boosting Activity and Stability of Metal Single-Atom Catalysts via Regulation of Coordination Number and Local Composition, Journal of the American Chemical Society, 143 (2021) 18854-18858.

[19] H. Tan, C. Wang, H.L. Duan, J. Tian, Q.Q. Ji, Y. Lu, F.C. Hu, W. Hu, G.N. Li, N. Li, Y. Wang, W.S. Chu, Z.H. Sun, W.S. Yan, Intrinsic Room-Temperature Ferromagnetism in V2C MXene Nanosheets, Acs Applied Materials & Interfaces, 13 (2021) 33363-33370.

[20] Y. Pan, L.X. Xu, L. Huang, W.X. He, H.M. Li, S.Y. Wang, Z.X. Long, Z.H. Sun, Identification of Active Sites in Pt-Co Bimetallic Catalysts for CO Oxidation, Acs Applied Energy Materials, 4 (2021) 11151-11161.

[21] Z.X. Long, C.C. Ao, L. Huang, W. Zhang, C.Y. Liu, L.D. Zhang, W.X. He, S.Y. Wang, Y. Pan, Z.H. Sun, Unique Coordination Structure of Cobalt Single-Atom Catalyst Supported on Dopant-Free Carbon, J. Phys. Chem. C, 125 (2021) 6735-6742.

[22] W. Hu, C. Wang, H. Tan, H.L. Duan, G.N. Li, N. Li, Q.Q. Ji, Y. Lu, Y. Wang, Z.H. Sun, F.C. Hu, W.S. Yan, Embedding atomic cobalt into graphene lattices to activate room-temperature ferromagnetism, Nature Communications, 12 (2021) 1854.

[23] W.X. He, L. Huang, C.Y. Liu, S.Y. Wang, Z.X. Long, F.C. Hu, Z.H. Sun, Interfacial sites in platinum-hydroxide-cobalt hybrid nanostructures for promoting CO oxidation activity, Nanoscale, 13 (2021) 2593-2600.

[24] J. Gu, M.Z. Jian, L. Huang, Z.H. Sun, A.W. Li, Y. Pan, J.Z. Yang, W. Wen, W. Zhou, Y. Lin, H.J. Wang, X.Y. Liu, L.L. Wang, X.X. Shi, X.H. Huang, L.N. Cao, S. Chen, X.S. Zheng, H.B. Pan, J.F. Zhu, S.Q. Wei, W.X. Li, J.L. Lu, Synergizing metal-support interactions and spatial confinement boosts dynamics of atomic nickel for hydrogenations, Nature Nanotechnology, 16 (2021) 1141-1153.

[25] H.L. Duan, C. Wang, G.N. Li, H. Tan, W. Hu, L. Cai, W. Liu, N. Li, Q.Q. Ji, Y. Wang, Y. Lu, W.S. Yan, F.C. Hu, W.H. Zhang, Z.H. Sun, Z.M. Qi, L. Song, S.Q. Wei, Single-Atom-Layer Catalysis in a MoS2 Monolayer Activated by Long-Range Ferromagnetism for the Hydrogen Evolution Reaction: Beyond Single-Atom Catalysis, Angew. Chem. Int. Ed., 60 (2021) 7251-7258.

[26] L. Cai, H.L. Duan, Q.H. Liu, C. Wang, H. Tan, W. Hu, F.C. Hu, Z.H. Sun, W.S. Yan, Ultrahigh-temperature ferromagnetism MoS2 Moire superlattice/graphene hybrid heterostructures, Nano Research, 14 (2021) 4182-4187.

[27] Z.L. Wang, J. Choi, M.Q. Xu, X.F. Hao, H. Zhang, Z. Jiang, M. Zuo, J. Kim, W. Zhou, X.G. Meng, Q. Yu, Z.H. Sun, S.Q. Wei, J.H. Ye, G.G. Wallace, D.L. Officer, Y. Yamauchi, Optimizing Electron Densities of Ni-N-C Complexes by Hybrid Coordination for Efficient Electrocatalytic CO2 Reduction, Chemsuschem, 13 (2020) 929-937.

[28] X.X. Shi, Y. Lin, L. Huang, Z.H. Sun, Y. Yang, X.H. Zhou, E. Vovk, X.Y. Liu, X.H. Huang, M. Sun, S.Q. Wei, J.L. Lu, Copper Catalysts in Semihydrogenation of Acetylene: From Single Atoms to Nanoparticles, Acs Catalysis, 10 (2020) 3495-3504.

[29] X.L. Mou, D.H. Wang, X.K. Liu, W. Liu, L.L. Cao, T. Yao, XAFS study on single-atomic-site Cu-1/N-graphene catalyst for oxygen reduction reaction, Radiat. Phys. Chem., 175 (2020) 108230.

[30] N. Li, H. Tan, X. Ding, H.L. Duan, W. Hu, G.N. Li, Q.Q. Ji, Y. Lu, Y. Wang, F.C. Hu, C. Wang, W.R. Cheng, Z.H. Sun, W.S. Yan, Phase-mediated robust interfacial electron-coupling over core-shell Co@carbon towards superior overall water splitting, Applied Catalysis B-Environmental, 266 (2020) 118621.

[31] Q.Q. Ji, Y. Kong, C. Wang, H. Tan, H.L. Duan, W. Hu, G.N. Li, Y. Lu, N. Li, Y. Wang, J. Tian, Z.M. Qi, Z.H. Sun, F.C. Hu, W.S. Yan, Lattice Strain Induced by Linker Scission in Metal-Organic Framework Nanosheets for Oxygen Evolution Reaction, Acs Catalysis, 10 (2020) 5691-5697.

[32] L. Huang, X.Y. Song, Y. Lin, C.Y. Liu, W.X. He, S.Y. Wang, Z.X. Long, Z.H. Sun, In situ observations of the structural dynamics of platinum-cobalt-hydroxide nanocatalysts under CO oxidation, Nanoscale, 12 (2020) 3273-3283.

[33] S. Fang, X.R. Zhu, X.K. Liu, J. Gu, W. Liu, D.H. Wang, W. Zhang, Y. Lin, J.L. Lu, S.Q. Wei, Y.F. Li, T. Yao, Uncovering near-free platinum single-atom dynamics during electrochemical hydrogen evolution reaction, Nature Communications, 11 (2020).

[34] H.L. Duan, W. Liu, P. Guo, F.M. Tang, W.S. Yan, T. Yao, Identifying the single active site in MoS2-based hydrogen evolution electrocatalyst by XAFS technique, Radiat. Phys. Chem., 175 (2020) 108151.

[35] S. Chen, L. Huang, Z.H. Sun, L.N. Cao, W.X. Ying, X.X. Shi, W. Liu, J. Gu, X.S. Zheng, J. Zhu, Y. Lin, S.Q. Wei, J.L. Lu, Synthesis of Quasi-Bilayer Subnano Metal-Oxide Interfacial Cluster Catalysts for Advanced Catalysis, Small, 16 (2020).

[36] H.W. Wang, Q.Q. Luo, W. Liu, Y. Lin, Q.Q. Guan, X.S. Zheng, H.B. Pan, J.F. Zhu, Z.H. Sun, S.Q. Wei, J.L. Yang, J.L. Lu, Quasi Pd1Ni single-atom surface alloy catalyst enables hydrogenation of nitriles to secondary amines, Nature Communications, 10 (2019) 4998.

[37] X.Y. Song, L. Huang, W.X. He, C.Y. Liu, F.C. Hu, Y. Jiang, Z.H. Sun, S.Q. Wei, Electronic Metal-Support Interactions between Pt Nanoparticles and Co(OH)(2) Flakes for CO Oxidation, J. Phys. Chem. C, 123 (2019) 10907-10916.

[38] Y. Meng, L. Sun, J. Gao, W. Tan, C. Chen, J. Yi, H.J.M. Bouwmeester, Z. Sun, K.S. Brinkman, Insights into the CO2 Stability-Performance Trade-Off of Antimony-Doped SrFeO3−δ Perovskite Cathode for Solid Oxide Fuel Cells, ACS Applied Materials & Interfaces, (2019).

[39] J.J. Li, Q.Q. Guan, H. Wu, W. Liu, Y. Lin, Z.H. Sun, X.X. Ye, X.S. Zheng, H.B. Pan, J.F. Zhu, S. Chen, W.H. Zhang, S.Q. Wei, J.L. Lu, Highly Active and Stable Metal Single-Atom Catalysts Achieved by Strong Electronic Metal-Support Interactions, Journal of the American Chemical Society, 141 (2019) 14515-14519.

[40] G.N. Li, H.L. Duan, W.R. Cheng, C. Wang, W. Hu, Z.H. Sun, H. Tan, N. Li, Q.Q. Ji, Y. Wang, Y. Lu, W.S. Yan, Interlayer Photoelectron Transfer Boosted by Bridged Ru-IV Atoms in GaS Nanosheets for Efficient Water Splitting, ACS Applied Materials & Interfaces, 11 (2019) 45561-45567.

[41] X. Kang, L. Huang, W. Liu, L. Xiong, Y. Pei, Z.H. Sun, S.X. Wang, S.Q. Wei, M.Z. Zhu, Reversible nanocluster structure transformation between face-centered cubic and icosahedral isomers, Chem. Sci., 10 (2019) 8685-8693.

[42] X.H. Huang, H. Yan, L. Huang, X.H. Zhang, Y. Lin, J.J. Li, Y.J. Xia, Y.F. Ma, Z.H. Sun, S.G. Wei, J.L. Lu, Toward Understanding of the Support Effect on Pd-1 Single-Atom-Catalyzed Hydrogenation Reactions, J. Phys. Chem. C, 123 (2019) 7922-7930.

[43] W. Hu, H. Tan, H. Duan, G. Li, N. Li, Q. Ji, Y. Lu, Y. Wang, Z. Sun, F. Hu, C. Wang, W. Yan, Synergetic Effect of Substitutional Dopants and Sulfur Vacancy in Modulating the Ferromagnetism of MoS2 Nanosheets, ACS Appl Mater Interfaces, 11 (2019) 31155-31161.

[44] H.L. Duan, P. Guo, C. Wang, H. Tan, W. Hu, W.S. Yan, C. Ma, L. Cai, L. Song, W.H. Zhang, Z.H. Sun, L.J. Wang, W.B. Zhao, Y.W. Yin, X.G. Li, S.Q. Wei, Beating the exclusion rule against the coexistence of robust luminescence and ferromagnetism in chalcogenide monolayers, Nature Communications, 10 (2019) 1584.

[45] W.R. Cheng, X. Zhao, H. Su, F.M. Tang, W. Che, H. Zhang, Q.H. Liu, Lattice-strained metal-organic-framework arrays for bifunctional oxygen electrocatalysis, Nature Energy, 4 (2019) 115-122.

[46] L.N. Cao, W. Liu, Q.Q. Luo, R.T. Yin, B. Wang, J. Weissenrieder, M. Soldemo, H. Yan, Y. Lin, Z.H. Sun, C. Ma, W.H. Zhang, S. Chen, H.W. Wang, Q.Q. Guan, T. Yao, S.Q. Wei, J.L. Yang, J.L. Lu, Atomically dispersed iron hydroxide anchored on Pt for preferential oxidation of CO in H-2, Nature, 565 (2019) 631-635.

 

招生信息

欢迎化学、材料、物理等相关专业，对科学研究有浓厚兴趣并有志从事科研工作的同学报考本课题组研究生。